{"id":2157,"date":"2025-08-16T10:01:10","date_gmt":"2025-08-16T10:01:10","guid":{"rendered":"https:\/\/www.europesays.com\/ie\/2157\/"},"modified":"2025-08-16T10:01:10","modified_gmt":"2025-08-16T10:01:10","slug":"observing-the-dynamics-of-quantum-states-generated-inside-nonlinear-optical-cavities","status":"publish","type":"post","link":"https:\/\/www.europesays.com\/ie\/2157\/","title":{"rendered":"Observing the dynamics of quantum states generated inside nonlinear optical cavities"},"content":{"rendered":"<p>Experimental setup<\/p>\n<p>Here, we briefly introduce our experimental setup. More detailed description of the setup can be found in the Supplementary Note\u00a0<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"supplementary material anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-63035-8#MOESM1\" rel=\"nofollow noopener\" target=\"_blank\">4<\/a>.<\/p>\n<p>Laser<\/p>\n<p>For the laser system, a Toptica FemtoFiber ultra 780 was customized to provide dual-wavelength femtosecond pulses, with 780\u2009nm and 1560\u2009nm. A total of 780\u2009nm signal is used to pump the OPO, and 1560\u2009nm signal is split into two different lines, one is the bias field and the other is the local oscillator (LO) that is used to measure the phase of the OPO steady-state. Pump and bias field have the same polarization state, and they are orthogonal to the polarization of the LO signal.<\/p>\n<p>OPO<\/p>\n<p>The OPO consists of a MgO:PPLN crystal (MSHG1550-0.5-1, Covesion Ltd., United Kingdom) in a free-space bow tie optical cavity. The crystal is placed on the oven mount (PV10, Covesion Ltd., United Kingdom), which is connected to the temperature controller (OC2, Covesion Ltd., United Kingdom). The cavity length is matched to a single round trip of the laser pulse, and stabilized by detecting the power of the out-coupled sum-frequency mixed signal between the pump and the OPO signal<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 40\" title=\"Cheng, Y., McCracken, R. &amp; Reid, D. Dither-free stabilization of a femtosecond doubly resonant OPO using parasitic sum-frequency mixing. Opt. Lett. 45, 768&#x2013;771 (2020).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-63035-8#ref-CR40\" id=\"ref-link-section-d111712294e2141\" rel=\"nofollow noopener\" target=\"_blank\">40<\/a>. The out-coupled sum-frequency mixed signal passes a narrow-band pass filter, which gives a linear change in the detected signal power as the cavity length deviates from the degenerate mode. A photodetector measures this error signal and a proportional-integral-derivative controller yields a voltage feedback to the piezoelectric actuator (PA44M3KW, Thorlabs, USA) attached to one of the cavity mirrors. To collect the statistics of the OPO steady-state and measure the probability, we modulate the pump and the bias signal at 10\u2009kHz using a lithium niobate electro-optic modulators (EO-AM-NR-C1, EO-AM-NR-C3, Thorlabs, USA for amplitude modulation, and EO-PM-NR-C1, EO-PM-NR-C3, Thorlabs, USA for phase modulation). The cavity lifetime is calculated from the loss of the OPO signal from each cavity mirror, which gives \u00a0~300\u2009ns.<\/p>\n<p>Preparing bias signal<\/p>\n<p>To match the temporal alignment between pump and bias pulses, we use an optical delay line with a linear translational stage. Additional precision could be achieved by using an electronically controlled motorized actuator (PIA25, Thorlabs, USA). To attenuate the bias signal before entering to the cavity, the bias field first passes a series of neutral density filters (NDC-100S-4, Thorlabs, USA). Then we use a combination of waveplates and polarizers to further attenuate the bias field. The last waveplate is mounted on a motorized precision rotation stage (KPRM1E\/M, Thorlabs, USA) which can be electronically controlled.<\/p>\n<p>Measuring bias field<\/p>\n<p>Because the bias pulse entering the cavity contains less than a few photons, we use the following protocol to measure the amplitude of the bias field. First, we place the power meter after the last polarizer and set the waveplate angle that gives the maximum bias power P0. Then the bias power at waveplate angle \u03d5 would be written as \\(P={P}_{0}{\\cos }^{2}(2(\\phi -{\\phi }_{0}))\\), where \u03d50 is the angle that gives the maximum power. We rotate the angle of the waveplate to sweep the bias field and measure the bias\u2013probability curve. After passing the last polarizer, we calculate the actual bias power that interacts inside the crystal, considering all the possible power loss happening at each optical component before it reaches at the crystal. The loss of each element is obtained either from our previous measurements<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 25\" title=\"Roques-Carmes, C. et al. Biasing the quantum vacuum to control macroscopic probability distributions. Science 381, 205&#x2013;209 (2023).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-63035-8#ref-CR25\" id=\"ref-link-section-d111712294e2259\" rel=\"nofollow noopener\" target=\"_blank\">25<\/a> or the manufacturer. Then we calculate the bias field \\(b=\\frac{{E}_{{{{{\\rm{bias,mean}}}}}}}{{T}_{{{{{\\rm{rt}}}}}}}\\sqrt{\\frac{\\epsilon V}{\\hslash {\\omega }_{0}}}\\). Ebias,mean is the mean electric field of the bias, Trt is the round trip time of the cavity, \u03f5 is the electric permittivity of the MgO:PPLN crystal, V is the mode volume, and \u03c90 is the angular frequency of the bias field. We use pulse duration of 190\u2009ns, beam waist of 10\u2009\u03bcm to calculate Ebias,mean and V<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 25\" title=\"Roques-Carmes, C. et al. Biasing the quantum vacuum to control macroscopic probability distributions. Science 381, 205&#x2013;209 (2023).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-63035-8#ref-CR25\" id=\"ref-link-section-d111712294e2379\" rel=\"nofollow noopener\" target=\"_blank\">25<\/a>.<\/p>\n<p>Although we initially estimated the bias field by measuring the power loss at each optical element, more precise calibration of the bias field can be achieved by measuring the bias\u2013probability relationship of the quantum vacuum state. Details of the calibration method can be found in the Supplementary Note\u00a0<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"supplementary material anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-63035-8#MOESM1\" rel=\"nofollow noopener\" target=\"_blank\">4<\/a>.<\/p>\n<p>Measuring the statistics of the OPO steady-states<\/p>\n<p>The sampled OPO signal and the LO are combined in a standard interferometry setup to measure the phase of the OPO steady-state. The polarization states of the OPO signal and the LO are matched before they are combined with the beam splitter cube. We add an additional delay stage on the LO line, using the same module that we used to control the temporal alignment between the pump and the bias pulses. Using the one output arm of the beam splitter, we check the temporal alignment between the OPO signal and the LO by observing the inference pattern with the camera (CMLN-13S2M-CS, Edmund Optics, USA). For the other arm, we measure the interference pattern with the photodetector (PDA50B2, Thorlabs, USA). The detected signal was recorded on the oscilloscope, collecting either 1000 (Fig.\u00a0<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"figure anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-63035-8#Fig2\" rel=\"nofollow noopener\" target=\"_blank\">2<\/a>) or 10,000 OPO steady-states (Fig.\u00a0<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"figure anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-63035-8#Fig3\" rel=\"nofollow noopener\" target=\"_blank\">3<\/a>) to measure the probability at a given bias field. The probability is defined as the number of steady-states with phase 0 rad divided by the number of total steady-states measured with the oscilloscope<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 41\" title=\"Roques-Carmes, C., Seouchoikr &amp; JamisonSloan. charlesrc\/pbit-opo: first release (original). Zenodo &#010;                  https:\/\/doi.org\/10.5281\/zenodo.7972106&#010;                  &#010;                 (2023).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-63035-8#ref-CR41\" id=\"ref-link-section-d111712294e2403\" rel=\"nofollow noopener\" target=\"_blank\">41<\/a>.<\/p>\n<p>Reconstruction protocol<\/p>\n<p>In this section, we describe some mathematical background on our Husimi Q function reconstruction protocol by measuring the sensitivity of the bias\u2013probability relationship.<\/p>\n<p>Husimi Q function<\/p>\n<p>The Husimi Q function gives the probability of observing a certain coherent state \\(\\left\\vert \\alpha \\right\\rangle\\) for a given quantum state \\(\\left\\vert \\psi \\right\\rangle\\):<\/p>\n<p>$$Q(\\alpha,{\\alpha }^{*})\t=\\frac{1}{\\pi }\\left\\langle \\alpha | \\rho | \\alpha \\right\\rangle \\\\ \t=\\frac{1}{\\pi }| \\left\\langle \\alpha | \\psi \\right\\rangle {| }^{2}.$$<\/p>\n<p>\n                    (2)\n                <\/p>\n<p>The Husimi Q function can be either reconstructed with a standard homodyne detection setup that combines the unknown quantum state \\(\\left\\vert \\psi \\right\\rangle\\) with a reference coherent state \\(\\left\\vert \\alpha \\right\\rangle\\)<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 42\" title=\"Nehra, R. et al. Generalized overlap quantum state tomography. Phys. Rev. Res. 2, 042002 (2020).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-63035-8#ref-CR42\" id=\"ref-link-section-d111712294e2655\" rel=\"nofollow noopener\" target=\"_blank\">42<\/a> or directly measured by using a heterodyne setup<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 43\" title=\"Stenholm, S. Simultaneous measurement of conjugate variables. Ann. Phys. 218, 233&#x2013;254 (1992).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-63035-8#ref-CR43\" id=\"ref-link-section-d111712294e2659\" rel=\"nofollow noopener\" target=\"_blank\">43<\/a>, which is also known as a double homodyne setup. We rewrite Eq. (<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"equation anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-63035-8#Equ2\" rel=\"nofollow noopener\" target=\"_blank\">2<\/a>) using the displacement operator D(\u03b1):<\/p>\n<p>$$Q(\\alpha,{\\alpha }^{*})\t \\equiv \\frac{1}{\\pi }| \\left\\langle \\alpha | \\psi \\right\\rangle {| }^{2}\\\\ \t=\\frac{1}{\\pi }| \\left\\langle 0| D(-\\alpha )| \\psi \\right\\rangle {| }^{2}.$$<\/p>\n<p>\n                    (3)\n                <\/p>\n<p>Equation (<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"equation anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-63035-8#Equ3\" rel=\"nofollow noopener\" target=\"_blank\">3<\/a>) shows that measuring the Husimi Q function is equivalent to measuring the overlap between the displaced quantum state \\(D(-\\alpha )\\left\\vert \\psi \\right\\rangle\\) and quantum vacuum state \\(\\left\\vert 0\\right\\rangle\\).<\/p>\n<p>Displacement operator<\/p>\n<p>The stochastic differential equation of the OPO signal defined along the real quadrature of the phase space X can be written as below<a data-track=\"click\" data-track-action=\"reference anchor\" data-track-label=\"link\" data-test=\"citation-ref\" aria-label=\"Reference 25\" title=\"Roques-Carmes, C. et al. Biasing the quantum vacuum to control macroscopic probability distributions. Science 381, 205&#x2013;209 (2023).\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-63035-8#ref-CR25\" id=\"ref-link-section-d111712294e2911\" rel=\"nofollow noopener\" target=\"_blank\">25<\/a>:<\/p>\n<p>$$\\dot{X}=(\\lambda -1)X+\\sqrt{2}b+\\sqrt{\\lambda }{\\eta }_{X}.$$<\/p>\n<p>\n                    (4)\n                <\/p>\n<p>Here, \u03b7X is the Gaussian noise. Because the derivative of the drift term \\((\\lambda -1)X+\\sqrt{2}b\\) with respect to X is positive when the OPO is pumped above threshold (i.e., \u03bb\u2009&gt;\u20091), the sign of the drift term at the time when the bias field is injected determines whether X will grow exponentially toward positive or negative side. Therefore, the direction of the amplification can be determined by the sign of the drift term. The critical point X0 with zero drift happens at \\({X}_{0}=-\\sqrt{2}b\/(\\lambda -1)\\). X0\u2009=\u20090 for an unbiased OPO, meaning that the amplification behavior of the cavity quantum state \\(\\left\\vert \\psi \\right\\rangle\\) in the biased OPO is identical to that of displaced quantum state \\(D(b)\\left\\vert \\psi \\right\\rangle\\) in the unbiased OPO, where the displacement operator D(b) defined along the X quadrature is written as:<\/p>\n<p>$$D(b)\\equiv \\frac{\\sqrt{2}b}{\\lambda -1}.$$<\/p>\n<p>\n                    (5)\n                <\/p>\n<p>Reconstructing marginal distribution of the Husimi Q function<\/p>\n<p>After the bias field displaces the quantum state, the OPO signal is amplified until it reaches one of the steady-states. As we described in the previous section, the original quantum state \\(\\left\\vert \\psi \\right\\rangle\\) in the biased OPO shows the same dynamics as \\(D(b)\\left\\vert \\psi \\right\\rangle\\) in the unbiased OPO system. The parametric amplification process is phase-sensitive, so X\u2009&gt;\u20090 (or equivalently Re(\u03b1)\u2009&gt;\u20090) part of the displaced quantum state gives the probability p of measuring a certain steady-state, which can be analytically described as:<\/p>\n<p>$$p(b| \\theta )\\equiv \\int_{\\alpha=0}^{\\alpha=\\infty }| {\\psi }_{\\theta,D(b)}(\\alpha ){| }^{2}d\\alpha,$$<\/p>\n<p>\n                    (6)\n                <\/p>\n<p>where \\(\\left\\vert {\\psi }_{\\theta,D(b)}\\right\\rangle \\equiv D(b)\\left\\vert {\\psi }_{\\theta }\\right\\rangle\\). Because the phase-sensitive amplification happens along one quadrature, we consider the marginal distribution \\(\\left\\vert {\\psi }_{\\theta }\\right\\rangle\\). Using basic algebra,<\/p>\n<p>$$p(b| \\theta )\t \\equiv \\int_{-D(b)}^{\\infty }| {\\psi }_{\\theta }(\\alpha ){| }^{2}d\\alpha \\\\ \t={\\left\\langle {\\psi }_{\\theta }| {\\psi }_{\\theta }\\right\\rangle }_{[-D(b),\\infty ]}\\\\ \t={\\left\\langle {\\psi }_{\\theta }| I| {\\psi }_{\\theta }\\right\\rangle }_{[-D(b),\\infty ]}\\\\ \t=\\frac{1}{\\pi }\\int| \\left\\langle {\\psi }_{\\theta }| \\alpha \\right\\rangle {| }_{[-D(b),\\infty ]}^{2}\\,{d}^{2}\\alpha \\\\ \t=\\int_{-D(b)}^{\\infty }\\int_{-\\infty }^{\\infty }Q\\,\\,{\\mbox{dIm}}({\\alpha }_{\\theta }){\\mbox{dRe}}\\,({\\alpha }_{\\theta }).$$<\/p>\n<p>\n                    (7)\n                <\/p>\n<p>We introduced the identity operator \\(I=\\frac{1}{\\pi }\\int\\left\\vert \\alpha \\right\\rangle \\left\\langle \\alpha \\right\\vert {{\\mbox{d}}}^{2}\\alpha\\), to expand the representation from a specific coordinate to the 2D phase space. The final expression represents the same probability but now sums over the possible coherent states in the region of interest. Therefore, by taking the derivative with respect to D(b), we can reconstruct the marginal distribution Q\u03b8.<\/p>\n<p>Stochastic differential equations<\/p>\n<p>Until now, we have focused on using the displacement operator to understand how the bias field b affects the probability p. In this section, we provide another approach, which solves the SDE of the OPO system to calculate the bias\u2013probability relationship. When a time-dependent bias field b(\u03c4) is introduced, the OPO dynamics at the linear amplification stage can be written as:<\/p>\n<p>$$\\dot{X}=(\\lambda -1)X+\\sqrt{2}b(\\tau )+\\sqrt{\\lambda }{\\eta }_{X}.$$<\/p>\n<p>\n                    (8)\n                <\/p>\n<p>With Z\u2009=\u2009Xe\u2212(\u03bb\u22121)\u03c4,<\/p>\n<p>$$Z(\\tau )=Z(0)+\\int_{0}^{\\tau }{e}^{-(\\lambda -1)\\tau {\\prime} }[\\sqrt{2}b(\\tau {\\prime} )+\\sqrt{\\lambda }{\\eta }_{X}(\\tau {\\prime} )]d\\tau {\\prime} .$$<\/p>\n<p>\n                    (9)\n                <\/p>\n<p>Calculating the positive area of the probability distribution of Z(\u03c4), we can calculate the probability p. When a constant bias field b0 is injected at \u03c4\u2009=\u2009\u03c40,<\/p>\n<p>$$P[Z(\\tau )\\ge 0]=P\\left[f(\\tau )\\ge -\\frac{\\sqrt{2}{b}_{0}}{\\sqrt{\\lambda }}\\frac{{e}^{-(\\lambda -1){\\tau }_{0}}-{e}^{-(\\lambda -1)\\tau }}{\\lambda -1}\\right],$$<\/p>\n<p>\n                    (10)\n                <\/p>\n<p>$$f(\\tau )\\equiv \\int_{0}^{\\tau }{e}^{-(\\lambda -1)\\tau {\\prime} }{\\eta }_{X}(\\tau {\\prime} )d\\tau {\\prime}$$<\/p>\n<p>\n                    (11)\n                <\/p>\n<p>Because X(\u03c4) is the Wiener process (linear superposition of Gaussian noises), f(\u03c4) is a Gaussian with mean \u3008f(\u03c4)\u3009\u2009=\u20090, and variance \\(\\langle \\,{f}^{2}(\\tau )\\rangle=\\frac{1-{e}^{-2(\\lambda -1)\\tau }}{2(\\lambda -1)}\\). Therefore,<\/p>\n<p>$$P[Z(\\tau )\\ge 0]=\\int_{-{f}_{0}(\\tau )}^{\\infty }\\frac{1}{\\sqrt{2\\pi \\langle \\,{f}^{2}(\\tau )\\rangle }}{e}^{-\\frac{{f}^{2}}{2\\langle \\,{f}^{2}(\\tau )\\rangle }}df,$$<\/p>\n<p>\n                    (12)\n                <\/p>\n<p>where \\({f}_{0}(\\tau )\\equiv \\frac{\\sqrt{2}{b}_{0}}{\\sqrt{\\lambda }}\\frac{{e}^{-(\\lambda -1){\\tau }_{0}}-{e}^{-(\\lambda -1)\\tau }}{\\lambda -1}\\). As we measure the probability p after several cavity cycles, which corresponds to the time \u03c4 when e\u2212(\u03bb\u22121)\u03c4\u2009\u2192\u20090+, so the probability p becomes<\/p>\n<p>$$p\\equiv P[Z(\\tau )\\ge 0]=\\frac{1}{2}\\left(1+\\,{\\mbox{erf}}\\,\\left[\\frac{\\sqrt{2}{b}_{0}{e}^{-(\\lambda -1){\\tau }_{0}}}{\\sqrt{\\lambda }\\sqrt{\\lambda -1}}\\right]\\right),$$<\/p>\n<p>\n                    (13)\n                <\/p>\n<p>where erf is the Gauss error function. In the Supplementary Information\u00a0<a data-track=\"click\" data-track-label=\"link\" data-track-action=\"supplementary material anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-63035-8#MOESM1\" rel=\"nofollow noopener\" target=\"_blank\">3<\/a> and <a data-track=\"click\" data-track-label=\"link\" data-track-action=\"supplementary material anchor\" href=\"http:\/\/www.nature.com\/articles\/s41467-025-63035-8#MOESM1\" rel=\"nofollow noopener\" target=\"_blank\">5<\/a>, we discuss the SDEs for time-dependent \u03bb(\u03c4) and b(\u03c4).<\/p>\n","protected":false},"excerpt":{"rendered":"Experimental setup Here, we briefly introduce our experimental setup. More detailed description of the setup can be found&hellip;\n","protected":false},"author":2,"featured_media":2158,"comment_status":"","ping_status":"","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[271],"tags":[18,1099,19,17,1100,2570,452,2571,133],"class_list":{"0":"post-2157","1":"post","2":"type-post","3":"status-publish","4":"format-standard","5":"has-post-thumbnail","7":"category-physics","8":"tag-eire","9":"tag-humanities-and-social-sciences","10":"tag-ie","11":"tag-ireland","12":"tag-multidisciplinary","13":"tag-nonlinear-optics","14":"tag-physics","15":"tag-quantum-optics","16":"tag-science"},"share_on_mastodon":{"url":"","error":""},"_links":{"self":[{"href":"https:\/\/www.europesays.com\/ie\/wp-json\/wp\/v2\/posts\/2157","targetHints":{"allow":["GET"]}}],"collection":[{"href":"https:\/\/www.europesays.com\/ie\/wp-json\/wp\/v2\/posts"}],"about":[{"href":"https:\/\/www.europesays.com\/ie\/wp-json\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"https:\/\/www.europesays.com\/ie\/wp-json\/wp\/v2\/users\/2"}],"replies":[{"embeddable":true,"href":"https:\/\/www.europesays.com\/ie\/wp-json\/wp\/v2\/comments?post=2157"}],"version-history":[{"count":0,"href":"https:\/\/www.europesays.com\/ie\/wp-json\/wp\/v2\/posts\/2157\/revisions"}],"wp:featuredmedia":[{"embeddable":true,"href":"https:\/\/www.europesays.com\/ie\/wp-json\/wp\/v2\/media\/2158"}],"wp:attachment":[{"href":"https:\/\/www.europesays.com\/ie\/wp-json\/wp\/v2\/media?parent=2157"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"https:\/\/www.europesays.com\/ie\/wp-json\/wp\/v2\/categories?post=2157"},{"taxonomy":"post_tag","embeddable":true,"href":"https:\/\/www.europesays.com\/ie\/wp-json\/wp\/v2\/tags?post=2157"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}