{"id":53290,"date":"2025-04-26T23:14:19","date_gmt":"2025-04-26T23:14:19","guid":{"rendered":"https:\/\/www.europesays.com\/uk\/53290\/"},"modified":"2025-04-26T23:14:19","modified_gmt":"2025-04-26T23:14:19","slug":"orbital-textures-and-evolution-of-correlated-insulating-state-in-monolayer-1t-phase-transition-metal-dichalcogenides","status":"publish","type":"post","link":"https:\/\/www.europesays.com\/uk\/53290\/","title":{"rendered":"Orbital textures and evolution of correlated insulating state in monolayer 1T phase transition metal dichalcogenides"},"content":{"rendered":"
  • \n

    Imada, M., Fujimori, A. & Tokura, Y. Metal-insulator transitions. Rev. Mod. Phys. 70<\/b>, 1039\u20131263 (1998).<\/p>\n

    Article<\/a>\u00a0
    \n     ADS<\/a>\u00a0
    \n     CAS<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Brandow, B. H. Electronic structure of Mott insulators. Adv. Phys. 26<\/b>, 652 (1977).<\/p>\n

    Article<\/a>\u00a0
    \n     ADS<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Mott, N. F. & Peierls, R. Discussion of the paper by de Boer and Verwey. Proc. Phys. Soc. 49<\/b>, 72\u201373 (1937).<\/p>\n

    Article<\/a>\u00a0
    \n     ADS<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Law, K. T. & Lee, P. A. 1T-TaS2 as a quantum spin liquid. Proc. Natl. Acad. Sci. USA 114<\/b>, 6996\u20137000 (2017).<\/p>\n

    Article<\/a>\u00a0
    \n     ADS<\/a>\u00a0
    \n     CAS<\/a>\u00a0
    \n     PubMed<\/a>\u00a0
    \n     PubMed Central<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Balents, L. Spin liquids in frustrated magnets. Nature 464<\/b>, 199\u2013208 (2010).<\/p>\n

    Article<\/a>\u00a0
    \n     ADS<\/a>\u00a0
    \n     CAS<\/a>\u00a0
    \n     PubMed<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Dagotto, E. Correlated electrons in high-temperature superconductors. Rev. Mod. Phys. 66<\/b>, 763\u2013840 (1994).<\/p>\n

    Article<\/a>\u00a0
    \n     ADS<\/a>\u00a0
    \n     CAS<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Lee, P. A., Nagaosa, N. & Wen, X. G. Doping a Mott insulator: physics of high-temperature superconductivity. Rev. Mod. Phys. 78<\/b>, 17\u201385 (2006).<\/p>\n

    Article<\/a>\u00a0
    \n     ADS<\/a>\u00a0
    \n     CAS<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Li, T. et al. Continuous Mott transition in semiconductor moire superlattices. Nature 597<\/b>, 350\u2013354 (2021).<\/p>\n

    Article<\/a>\u00a0
    \n     ADS<\/a>\u00a0
    \n     CAS<\/a>\u00a0
    \n     PubMed<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Chen, G. et al. Evidence of a gate-tunable Mott insulator in a trilayer graphene moir\u00e9 superlattice. Nat. Phys. 15<\/b>, 237 (2019).<\/p>\n

    Article<\/a>\u00a0
    \n     CAS<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Fath, M. et al. Spatially inhomogeneous metal-insulator transition in doped manganites. Science 285<\/b>, 1540 (1999).<\/p>\n

    Article<\/a>\u00a0
    \n     CAS<\/a>\u00a0
    \n     PubMed<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Chatzieleftheriou, M. et al. Mott quantum critical points at finite doping. Phys. Rev. Lett. 130<\/b>, 066401 (2023).<\/p>\n

    Article<\/a>\u00a0
    \n     ADS<\/a>\u00a0
    \n     CAS<\/a>\u00a0
    \n     PubMed<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Gelabert, M., Lachicotte, R. & DiSalvo, F. Insulator-metal and structural phase phenomena in KxBa1-xCoS2 (x Chem. Mater. 10<\/b>, 613\u2013619 (1998).<\/p>\n

    Article<\/a>\u00a0
    \n     CAS<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Di Salvo, F. J., Wilson, J. A., Bagley, B. G. & Waszczak, J. V. Effects of doping on charge-density waves in layer compounds. Phys. Rev. B 12<\/b>, 2220\u20132236 (1975).<\/p>\n

    Article<\/a>\u00a0
    \n     ADS<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Di Salvo, F. J., Maines, R. G., Waszczak, J. V. & Schwall, R. E. Preparation and properties of 1T-TaSe2. Solid State Commun. 14<\/b>, 497\u2013501 (1974).<\/p>\n

    Article<\/a>\u00a0
    \n     ADS<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Fazekas, P. & Tosatti, E. Electrical, structural and magnetic properties of pure and doped 1T-TaS2. Philoso. Mag. B 39<\/b>, 229\u2013244 (1979).<\/p>\n

    Article<\/a>\u00a0
    \n     ADS<\/a>\u00a0
    \n     CAS<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Colonna, S. et al. Mott phase at the surface of 1T-TaSe2 observed by scanning tunneling microscopy. Phys. Rev. Lett. 94<\/b>, 036405 (2005).<\/p>\n

    Article<\/a>\u00a0
    \n     ADS<\/a>\u00a0
    \n     PubMed<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Perfetti, L. et al. Spectroscopic signatures of a bandwidth-controlled Mott transition at the surface of 1T-TaSe2. Phys. Rev. Lett. 90<\/b>, 166401 (2003).<\/p>\n

    Article<\/a>\u00a0
    \n     ADS<\/a>\u00a0
    \n     CAS<\/a>\u00a0
    \n     PubMed<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Va\u0148o, V. et al. Artificial heavy fermions in a van der Waals heterostructure. Nature 599<\/b>, 582\u2013586 (2021).<\/p>\n

    Article<\/a>\u00a0
    \n     ADS<\/a>\u00a0
    \n     PubMed<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Lin, H. et al. Scanning tunneling spectroscopic study of monolayer 1T-TaS2 and 1T-TaSe2. Nano Res. 13<\/b>, 133\u2013137 (2020).<\/p>\n

    Article<\/a>\u00a0
    \n     CAS<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Chen, Y. et al. Strong correlations and orbital texture in single-layer 1T-TaSe2. Nat. Phys. 16<\/b>, 218 (2020).<\/p>\n

    Article<\/a>\u00a0
    \n     CAS<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Nakata, Y. et al. Robust charge-density wave strengthened by electron correlations in monolayer 1T-TaSe2 and 1T-NbSe2. Nat. Commun. 12<\/b>, 5873 (2021).<\/p>\n

    Article<\/a>\u00a0
    \n     ADS<\/a>\u00a0
    \n     CAS<\/a>\u00a0
    \n     PubMed<\/a>\u00a0
    \n     PubMed Central<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Zhang, H. et al. Impenetrable barrier at the Metal-Mott insulator junction in polymorphic 1H and 1T-NbSe2 lateral heterostructure. J. Phys. Chem. Lett. 13<\/b>, 10713 (2022).<\/p>\n

    Article<\/a>\u00a0
    \n     CAS<\/a>\u00a0
    \n     PubMed<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Ritschel, T. et al. Orbital textures and charge density waves in transition metal dichalcogenides. Nat. Phys. 11<\/b>, 328\u2013331 (2015).<\/p>\n

    Article<\/a>\u00a0
    \n     CAS<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Butler, C. J., Yoshida, M., Hanaguri, T. & Iwasa, Y. Mottness versus unit-cell doubling as the driver of the insulating state in 1T-TaS2. Nat. Commun. 11<\/b>, 2477 (2020).<\/p>\n

    Article<\/a>\u00a0
    \n     ADS<\/a>\u00a0
    \n     CAS<\/a>\u00a0
    \n     PubMed<\/a>\u00a0
    \n     PubMed Central<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Qiu, D. Y., Da Jornada, F. H. & Louie, S. G. Screening and many-body effects in two-dimensional crystals: monolayer MoS2. Phys. Rev. B 93<\/b>, 235435 (2016).<\/p>\n

    Article<\/a>\u00a0
    \n     ADS<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Halperin, B. I. & Rice, T. M. Possible anomalies at a semimetal-semiconductor transition. Rev. Mod. Phys. 40<\/b>, 755\u2013766 (1968).<\/p>\n

    Article<\/a>\u00a0
    \n     ADS<\/a>\u00a0
    \n     CAS<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Wang, Y. D. et al. Band insulator to Mott insulator transition in 1T-TaS2. Nat. Commun. 11<\/b>, 4215 (2020).<\/p>\n

    Article<\/a>\u00a0
    \n     ADS<\/a>\u00a0
    \n     CAS<\/a>\u00a0
    \n     PubMed<\/a>\u00a0
    \n     PubMed Central<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Wang, Y. et al. Dualistic insulator states in 1T-TaS2 crystals. Nat. Commun. 15<\/b>, 3425 (2024).<\/p>\n

    Article<\/a>\u00a0
    \n     ADS<\/a>\u00a0
    \n     CAS<\/a>\u00a0
    \n     PubMed<\/a>\u00a0
    \n     PubMed Central<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Calandra, M. Phonon-assisted magnetic Mott-insulating state in the charge density wave phase of single-layer 1T-NbSe2. Phys. Rev. Lett. 121<\/b>, 026401 (2018).<\/p>\n

    Article<\/a>\u00a0
    \n     ADS<\/a>\u00a0
    \n     CAS<\/a>\u00a0
    \n     PubMed<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Jiang, T. et al. Two-dimensional charge density wave TaX2 (X = S, Se, Te) from first principles. Phys. Rev. B 104<\/b>, 075147 (2021).<\/p>\n

    Article<\/a>\u00a0
    \n     ADS<\/a>\u00a0
    \n     CAS<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    He, W. Y. et al. Spinon fermi surface in a cluster Mott insulator model on a triangular lattice and possible application to 1T-TaS2. Phys. Rev. Lett. 121<\/b>, 046401 (2018).<\/p>\n

    Article<\/a>\u00a0
    \n     ADS<\/a>\u00a0
    \n     CAS<\/a>\u00a0
    \n     PubMed<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Chen, H. et al. Spectroscopic evidence for possible quantum spin liquid behavior in a two-dimensional Mott insulator. Phys. Rev. Lett. 134<\/b>, 066402 (2025).<\/p>\n

    Article<\/a>\u00a0
    \n     CAS<\/a>\u00a0
    \n     PubMed<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Norman, M. R., Randeria, M., Ding, H. & Campuzano, J. C. Phenomenology of the low-energy spectral function in high-TC superconductors. Phys. Rev. B 57<\/b>, R11093\u2013R11096 (1998).<\/p>\n

    Article<\/a>\u00a0
    \n     ADS<\/a>\u00a0
    \n     CAS<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Ohta, Y., Tohyama, T. & Maekawa, S. Apex oxygen and critical temperature in copper oxide superconductors: universal correlation with the stability of local singlets. Phys. Rev. B 43<\/b>, 2968\u20132982 (1991).<\/p>\n

    Article<\/a>\u00a0
    \n     ADS<\/a>\u00a0
    \n     CAS<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Slezak, J. A. et al. Imaging the impact on cuprate superconductivity of varying the interatomic distances within individual crystal unit cells. Proc. Natl. Acad. Sci. USA 105<\/b>, 3203\u20133208 (2008).<\/p>\n

    Article<\/a>\u00a0
    \n     ADS<\/a>\u00a0
    \n     CAS<\/a>\u00a0
    \n     PubMed<\/a>\u00a0
    \n     PubMed Central<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Weber, C., Haule, K. & Kotliar, G. Apical oxygens and correlation strength in electron- and hole-doped copper oxides. Phys. Rev. B 82<\/b>, 125107 (2010).<\/p>\n

    Article<\/a>\u00a0
    \n     ADS<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Hohenberg, P. & Kohn, W. Inhomogeneous electron gas. Phys. Rev. 136<\/b>, B864\u2013B871 (1964).<\/p>\n

    Article<\/a>\u00a0
    \n     ADS<\/a>\u00a0
    \n     MathSciNet<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Kresse, G. & Furthm\u00fcller, J. Efficiency of ab-initio total energy calculations for metals and semiconductors using a plane-wave basis set. Comput. Mater. Sci. 6<\/b>, 15\u201350 (1996).<\/p>\n

    Article<\/a>\u00a0
    \n     CAS<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Bl\u00f6chl, P. E. Projector augmented-wave method. Phys. Rev. B 50<\/b>, 17953\u201317979 (1994).<\/p>\n

    Article<\/a>\u00a0
    \n     ADS<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Perdew, J. P., Burke, K. & Ernzerhof, M. Generalized gradient approximation made simple. Phys. Rev. Lett. 77<\/b>, 3865\u20133868 (1996).<\/p>\n

    Article<\/a>\u00a0
    \n     ADS<\/a>\u00a0
    \n     CAS<\/a>\u00a0
    \n     PubMed<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Langreth, D. C. & Mehl, M. J. Beyond the local-density approximation in calculations of ground-state electronic properties. Phys. Rev. B 28<\/b>, 1809\u20131834 (1983).<\/p>\n

    Article<\/a>\u00a0
    \n     ADS<\/a>\u00a0
    \n     CAS<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Darancet, P., Millis, A. J. & Marianetti, C. A. Three-dimensional metallic and two-dimensional insulating behavior in octahedral tantalum dichalcogenides. Phys. Rev. B 90<\/b>, 045134 (2014).<\/p>\n

    Article<\/a>\u00a0
    \n     ADS<\/a>\u00a0
    \n     CAS<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n

  • \n

    Wang, V., Xu, N., Liu, J. C., Tang, G. & Geng, W. T. VASPKIT: a user-friendly interface facilitating high-throughput computing and analysis using VASP code. Comput. Phys. Commun. 267<\/b>, 108033 (2021).<\/p>\n

    Article<\/a>\u00a0
    \n     CAS<\/a>\u00a0
    \n
    \n Google Scholar<\/a>\u00a0\n <\/p>\n<\/li>\n","protected":false},"excerpt":{"rendered":"Imada, M., Fujimori, A. & Tokura, Y. Metal-insulator transitions. Rev. Mod. Phys. 70, 1039\u20131263 (1998). Article\u00a0 ADS\u00a0 CAS\u00a0…\n","protected":false},"author":2,"featured_media":53291,"comment_status":"","ping_status":"","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[3845],"tags":[20546,3965,17354,3966,74,70,17353,16,15],"class_list":{"0":"post-53290","1":"post","2":"type-post","3":"status-publish","4":"format-standard","5":"has-post-thumbnail","7":"category-physics","8":"tag-electronic-properties-and-materials","9":"tag-humanities-and-social-sciences","10":"tag-interfaces-and-thin-films","11":"tag-multidisciplinary","12":"tag-physics","13":"tag-science","14":"tag-surfaces","15":"tag-uk","16":"tag-united-kingdom"},"share_on_mastodon":{"url":"https:\/\/pubeurope.com\/@uk\/114406808847302987","error":""},"_links":{"self":[{"href":"https:\/\/www.europesays.com\/uk\/wp-json\/wp\/v2\/posts\/53290","targetHints":{"allow":["GET"]}}],"collection":[{"href":"https:\/\/www.europesays.com\/uk\/wp-json\/wp\/v2\/posts"}],"about":[{"href":"https:\/\/www.europesays.com\/uk\/wp-json\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"https:\/\/www.europesays.com\/uk\/wp-json\/wp\/v2\/users\/2"}],"replies":[{"embeddable":true,"href":"https:\/\/www.europesays.com\/uk\/wp-json\/wp\/v2\/comments?post=53290"}],"version-history":[{"count":0,"href":"https:\/\/www.europesays.com\/uk\/wp-json\/wp\/v2\/posts\/53290\/revisions"}],"wp:featuredmedia":[{"embeddable":true,"href":"https:\/\/www.europesays.com\/uk\/wp-json\/wp\/v2\/media\/53291"}],"wp:attachment":[{"href":"https:\/\/www.europesays.com\/uk\/wp-json\/wp\/v2\/media?parent=53290"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"https:\/\/www.europesays.com\/uk\/wp-json\/wp\/v2\/categories?post=53290"},{"taxonomy":"post_tag","embeddable":true,"href":"https:\/\/www.europesays.com\/uk\/wp-json\/wp\/v2\/tags?post=53290"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}