• Snaith, H. J. Present status and future prospects of perovskite photovoltaics. Nat. Mater. 17, 372–376 (2018).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Park, S. M. et al. Low-loss contacts on textured substrates for inverted perovskite solar cells. Nature 624, 289–294 (2023).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Lin, R. et al. All-perovskite tandem solar cells with improved grain surface passivation. Nature 603, 73–78 (2022).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Azmi, R. et al. Double-side 2D/3D heterojunctions for inverted perovskite solar cells. Nature 628, 93–98 (2024).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Shen, Z. et al. Precise synthesis of advanced polyarylamines for efficient perovskite solar cells. Nat. Mater. 24, 1450–1456 (2025).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Wang, Y. et al. Teaching an old anchoring group new tricks: enabling low-cost, eco-friendly hole-transporting materials for efficient and stable perovskite solar cells. J. Am. Chem. Soc. 142, 16632–16643 (2020).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • He, R. et al. Improving interface quality for 1-cm2 all-perovskite tandem solar cells. Nature 618, 80–86 (2023).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Zhao, K. et al. Peri-fused polyaromatic molecular contacts for perovskite solar cells. Nature 632, 301–306 (2024).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Al-Ashouri, A. et al. Conformal monolayer contacts with lossless interfaces for perovskite single junction and monolithic tandem solar cells. Energy Environ. Sci. 12, 3356–3369 (2019).

    Article 
    CAS 

    Google Scholar
     

  • Li, Z. et al. Stabilized hole-selective layer for high-performance inverted p–i–n perovskite solar cells. Science 382, 284–289 (2023).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Qu, G. et al. Conjugated linker-boosted self-assembled monolayer molecule for inverted perovskite solar cells. Joule 8, 2123–2134 (2024).

    Article 
    CAS 

    Google Scholar
     

  • Magomedov, A. et al. Self-assembled hole transporting monolayer for highly efficient perovskite solar cells. Adv. Energy Mater. 8, 1801892 (2018).

    Article 

    Google Scholar
     

  • Jiang, W. et al. π-Expanded carbazoles as hole-selective self-assembled monolayers for high-performance perovskite solar cells. Angew. Chem. Int. Ed. 134, e202213560 (2022).

    Article 

    Google Scholar
     

  • Paniagua, S. A. et al. Phosphonic acids for interfacial engineering of transparent conductive oxides. Chem. Rev. 116, 7117–7158 (2016).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Li, M., Liu, M., Qi, F., Lin, F. R. & Jen, A. K.-Y. Self-assembled monolayers for interfacial engineering in solution-processed thin-film electronic devices: design, fabrication, and applications. Chem. Rev. 124, 2138–2204 (2024).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Luo, C. et al. Engineering bonding sites enables uniform and robust self-assembled monolayer for stable perovskite solar cells. Nat. Mater. 24, 1265–1272 (2025).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Ji, X. et al. Efficient wide-bandgap perovskite solar cells with open-circuit voltage deficit below 0.4 V via hole-selective interface engineering. Sci. China Chem. 67, 2102–2110 (2024).

    Article 
    CAS 

    Google Scholar
     

  • Zhan, L., Zhang, L., Li, Y., Cai, H. & Wu, Y. Performance and stability enhancement of hole-transporting materials in inverted perovskite solar cells. ACS Appl. Energy Mater. 8, 3985–3996 (2025).

    Article 
    CAS 

    Google Scholar
     

  • Zhou, J. et al. Molecular contacts with an orthogonal π-skeleton induce amorphization to enhance perovskite solar cell performance. Nat. Chem. 17, 564–570 (2025).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Zhang, S. et al. Self-assembled π-conjugated hole-selective molecules for UV-resistant high-efficiency perovskite solar cells. Angew. Chem. Int. Ed. 64, e202508782 (2025).

    Article 
    CAS 

    Google Scholar
     

  • Li, C. et al. Fully aromatic self-assembled hole-selective layer toward efficient inverted wide-bandgap perovskite solar cells with ultraviolet resistance. Angew. Chem. Int. Ed. 63, e202315281 (2024).

    Article 
    CAS 

    Google Scholar
     

  • Wan, X. et al. Thermal stability of phosphonic acid self-assembled monolayers on alumina substrates. J. Phys. Chem. C 124, 2531–2542 (2020).

    Article 
    CAS 

    Google Scholar
     

  • Atanasov, V. et al. Synergistically integrated phosphonated poly(pentafluorostyrene) for fuel cells. Nat. Mater. 20, 370–377 (2021).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Fei, C. et al. Strong-bonding hole-transport layers reduce ultraviolet degradation of perovskite solar cells. Science 384, 1126–1134 (2024).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Luo, C. et al. Engineering the buried interface in perovskite solar cells via lattice-matched electron transport layer. Nat. Photon. 17, 856–864 (2023).

    Article 
    CAS 

    Google Scholar
     

  • Zhan, L. et al. Reinforced perovskite-substrate interfaces via multi-sited and dual-sided anchoring. Adv. Mater. 37, 2506048 (2025).

    Article 
    CAS 

    Google Scholar
     

  • Chen, X. et al. Studies on the effect of solvents on self-assembled monolayers formed from organophosphonic acids on indium tin oxide. Langmuir 28, 9487–9495 (2012).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Zhang, S. et al. Minimizing buried interfacial defects for efficient inverted perovskite solar cells. Science 380, 404–409 (2023).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Tang, H. et al. Reinforcing self-assembly of hole transport molecules for stable inverted perovskite solar cells. Science 383, 1236–1240 (2024).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Isikgor, F. H. et al. Molecular engineering of contact interfaces for high-performance perovskite solar cells. Nat. Rev. Mater. 8, 89–108 (2022).

    Article 

    Google Scholar
     

  • Jiang, W. et al. Toughened self-assembled monolayers for durable perovskite solar cells. Nature 646, 95–101 (2025).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Anderson, K. L. & Edwards, M. A. A tutorial for scanning electrochemical cell microscopy (SECCM) measurements: step-by-step instructions, visual resources, and guidance for first experiments. ACS Meas. Sci. Au 5, 160–177 (2025).

    Article 
    CAS 
    PubMed 
    PubMed Central 

    Google Scholar
     

  • Wu, W. et al. Stable and uniform self-assembled organic diradical molecules for perovskite photovoltaics. Science 389, 195–199 (2025).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Ulman, A. Formation and structure of self-assembled monolayers. Chem. Rev. 96, 1533–1554 (1996).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Zhang, S., Baker, J. & Pulay, P. A reliable and efficient first principles-based method for predicting pKa values. 1. Methodology. J. Phys. Chem. A 114, 425–431 (2010).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Liptak, M. D. & Shields, G. C. Accurate p Ka calculations for carboxylic acids using complete basis set and gaussian-n models combined with CPCM continuum solvation methods. J. Am. Chem. Soc. 123, 7314–7319 (2001).

    Article 
    CAS 
    PubMed 

    Google Scholar
     

  • Frisch, M. J., Head-Gordon, M. & Pople, J. A. A direct MP2 gradient method. Chem. Phys. Lett. 166, 275–280 (1990).

    Article 
    CAS 

    Google Scholar
     

  • Kresse, G. & Furthmüller, J. Efficient iterative schemes for ab initio total-energy calculations using a plane-wave basis set. Phys. Rev. B 54, 11169–11186 (1996).

    Article 
    CAS 

    Google Scholar
     

  • Blöchl, P. E. Projector augmented-wave method. Phys. Rev. B 50, 17953–17979 (1994).

    Article 

    Google Scholar
     

  • Goedecker, S., Teter, M. & Hutter, J. Separable dual-space Gaussian pseudopotentials. Phys. Rev. B 54, 1703–1710 (1996).

    Article 
    CAS 

    Google Scholar
     

  • Lee, K., Murray, ÉD., Kong, L., Lundqvist, B. I. & Langreth, D. C. Higher-accuracy van der Waals density functional. Phys. Rev. B 82, 081101 (2010).

    Article 

    Google Scholar